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Table A.1
Uncertainties ΔC from nuclear data libraries for the ENRESA samples for the isotopic concentrations (CASMO5-1 calculations). All values are in %. The last three columns present the maximum uncertainties (due to nuclear data) for the PWR samples GU1, GU3 and BM1 (BM1 being a MOX sample).
| ENRESA-1 | min-max(ENRESA-1 -8) ENDF/B-VIII.0 | GU1 (max) | GU3 (max) | BM1 (max) | |||
|---|---|---|---|---|---|---|---|
| ENDF/B-VIII.0 | JEFF-3.3 | JENDL-4.0 | |||||
| 234U | 1.9 | 2.0 | 7.3 | 1.4–2.2 | 9.9 | 7.9 | 4.5 |
| 235U | 1.6 | 2.1 | 2.5 | 0.9–2.6 | 4.1 | 1.8 | 1.1 |
| 236U | 0.7 | 1.7 | 1.2 | 0.7–0.8 | 1.6 | 1.7 | 1.7 |
| 238U | 0.0 | 0.0 | 0.0 | 0.0 | 0.0 | 0.0 | 0.0 |
| 237Np | 3.3 | 4.0 | 4.0 | 3.1–3.5 | – | 4.0 | 18 |
| 238Pu | 4.8 | 11 | 7.9 | 4.3–5.0 | 13 | 9.4 | 8.0 |
| 239Pu | 2.0 | 1.9 | 2.3 | 1.7–2.0 | 2.6 | 2.2 | 2.0 |
| 240Pu | 4.0 | 2.3 | 4.1 | 3.9–4.1 | 4.9 | 4.4 | 2.8 |
| 241Pu | 3.3 | 3.2 | 3.7 | 3.1–3.7 | 3.9 | 3.4 | 3.2 |
| 242Pu | 4.4 | 8.4 | 8.5 | 4.2–4.7 | 8.7 | 8.6 | 6.1 |
| 241Am | 3.5 | 3.3 | 4.1 | 3.2–3.7 | 4.4 | 3.9 | 3.6 |
| 243Am | 8.8 | 7.9 | 9.3 | 8.2–9.6 | 8.7 | 9.0 | 6.2 |
| 244Cm | 9.8 | 9.6 | 10 | 9.2–11 | 9.7 | 10 | 6.8 |
| 246Cm | 25 | 22 | 25 | 25–26 | 24 | 24 | 23 |
| 90Sr | 0.7 | 1.4 | 0.7 | 0.7–0.9 | 1.3 | 1.4 | 1.5 |
| 94Mo | 4.7 | 17 | 13 | 4.5–5.1 | – | – | – |
| 95Mo | 0.9 | 0.7 | 0.8 | 0.9 | 0.8 | 0.9 | 1.1 |
| 96Mo | 3.8 | 3.7 | 1.3 | 3.4–4.1 | – | – | – |
| 97Mo | 1.1 | 0.7 | 1.1 | 1.1–1.2 | – | – | – |
| 98Mo | 0.2 | 0.1 | 0.2 | 0.2–0.4 | – | – | – |
| 100Mo | 1.3 | 0.9 | 1.3 | 1.1–1.4 | – | – | – |
| 99Tc | 1.4 | 0.7 | 1.4 | 1.3–1.5 | 1.8 | 1.6 | 2.6 |
| 101Ru | 2.7 | 0.9 | 2.8 | 2.4–2.9 | 3.4 | 3.1 | 5.0 |
| 102Ru | 0.4 | 0.2 | 0.2 | 0.3–0.7 | – | – | – |
| 103Ru | 1.3 | 1.0 | 1.3 | 1.2–1.4 | – | – | – |
| 104Ru | 0.9 | 1.7 | 0.8 | 0.8–1.0 | – | – | – |
| 106Ru | 1.4 | 1.8 | 1.5 | 1.4–2.1 | 1.8 | 1.7 | 1.8 |
| 103Rh | 1.6 | 1.5 | 1.2 | 1.4–1.8 | 2.0 | 1.7 | 1.8 |
| 109Ag | 22 | 4.2 | 25 | 21–25 | 21 | 21 | 24 |
| 105Pd | 1.8 | 2.0 | 1.7 | 1.8–1.9 | – | – | – |
| 107Pd | 0.4 | 0.5 | 0.6 | 0.4–0.7 | – | – | – |
| 108Pd | 14 | 3.1 | 9.7 | 13–14 | – | – | – |
| 110Pd | 15 | 7.3 | 11 | 14–15 | – | – | – |
| 111Cd | 20 | 8.6 | 17 | 20–21 | – | – | – |
| 112Cd | 1.2 | 0.7 | 1.1 | 1.0–1.6 | – | – | – |
| 114Cd | 4.8 | 4.3 | 4.6 | 4.6–4.8 | – | – | – |
| 125Sb | 18 | 28 | 16 | 17–19 | – | 30 | 35 |
| 129 | 2.9 | 5.9 | 2.8 | 2.4–3.1 | – | 6.1 | – |
| 133Cs | 29 | 2.3 | 28 | 28–31 | 29 | 30 | – |
| 134Cs | 29 | 4.1 | 28 | 29–32 | 28 | 30 | – |
| 135Cs | 7.8 | 17 | 7.7 | 7.4–9.6 | 19 | 20 | – |
| 137Cs | 6.8 | 3.6 | 6.8 | 6.6–7.3 | 6.5 | 6.9 | – |
| 139La | 0.6 | 0.5 | 0.6 | 0.6–0.7 | – | – | – |
| 140Ce | 0.6 | 0.5 | 0.6 | 0.6–0.8 | – | – | – |
| 142Ce | 0.4 | 0.6 | 0.5 | 0.4–0.5 | – | – | - |
| 144Ce | 0.4 | 0.6 | 0.5 | 0.4–0.5 | 0.7 | 0.6 | 0.9 |
| 142Nd | 4.1 | 4.0 | 1.2 | 3.4–4.7 | 4.3 | 5.1 | 7.1 |
| 143Nd | 2.0 | 4.3 | 1.0 | 1.5–2.3 | 5.1 | 3.6 | 1.6 |
| 144Nd | 0.9 | 1.9 | 0.5 | 0.8–1.2 | 1.9 | 2.2 | 1.3 |
| 145Nd | 1.7 | 0.9 | 0.4 | 1.3–2.0 | 2.3 | 2.0 | 1.5 |
| 146Nd | 1.4 | 0.8 | 0.4 | 1.2–1.7 | 1.7 | 1.7 | 1.4 |
| 148Nd | 0.4 | 0.6 | 0.4 | 0.4–0.5 | 0.9 | 0.6 | 0.8 |
| 150Nd | 0.4 | 0.9 | 0.4 | 0.4–0.5 | 0.9 | 0.9 | 1.1 |
| 147Sm | 1.9 | 1.2 | 1.1 | 1.5–2.8 | 2.5 | 2.2 | 2.6 |
| 148Sm | 1.6 | 1.6 | 1.0 | 1.5–2.0 | 2.0 | 1.9 | 2.4 |
| 149Sm | 2.1 | 4.7 | 2.2 | 2.1–2.3 | 3.4 | 3.5 | 4.1 |
| 150Sm | 1.3 | 1.3 | 1.2 | 1.3–1.4 | 1.5 | 1.3 | 1.7 |
| 151Sm | 2.5 | 13 | 1.9 | 2.5–2.6 | 13 | 12 | 12 |
| 152Sm | 2.2 | 3.5 | 1.2 | 2.1–2.4 | 3.9 | 3.8 | 4.2 |
| 154Sm | 1.7 | 7.4 | 1.7 | 1.6–1.8 | 7.8 | 7.4 | 11 |
| 153Eu | 2.9 | 2.2 | 1.1 | 2.6–3.2 | 3.3 | 3.3 | 3.5 |
| 154Eu | 2.3 | 2.3 | 1.2 | 2.3–3.4 | 2.2 | 2.8 | 4.3 |
| 155Eu | 16 | 16 | 1.2 | 13–18 | 21 | 24 | 33 |
| 154Gd | 2.6 | 2.4 | 1.2 | 2.5–4.2 | – | – | 4.4 |
| 155Gd | 16 | 16 | 1.2 | 13–18 | 20 | 23 | 33 |
| 156Gd | 2.9 | 2.9 | 1.8 | 2.8–3.6 | – | – | 6.5 |
| 157Gd | 4.6 | 10 | 4.5 | 4.2–5.5 | – | – | – |
| 158Gd | 1.3 | 3.1 | 0.9 | 1.0–1.5 | – | – | 3.3 |
| 160Gd | 9.0 | 29 | 9.1 | 9.0–9.1 | – | – | 27 |
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