Open Access
Table A.2
Experimental and recommended values for fission products from the ARIANE report and reference [8]. Uncertainties correspond to 1σ. See text for details. Values with a * are given here at the date of measurements, whereas they are given at EOL in reference [8]. Values in mg/gU are used in this work.
| Measurement | Measurement | Recommendation | Recommendation | ||||||||
|---|---|---|---|---|---|---|---|---|---|---|---|
| GU3 (ITU) [5] | GU3’ (SCK) [5] | deduced from ORNL [8] | ARIANE [5] | ||||||||
| mg/gU | mg/gfuel | date | mg/gU | mg/gfuel | date | mg/gU | mg/gfuel | date | mg/gfuel | date | |
| 90Sr | 0.780 | 0.645 ± 0.32% | 07.10.99 | 0.763 | 0.630 ± 8.01% | 16.05.00 | 0.780* | 0.645* ± 0.32% | 07.10.99 | 0.683 ± 0.31% | EOL |
| 95Mo | 1.013 | 1.031 ± 0.51% | 19.11.99 | 1.39 | 1.147 ± 4.57% | 19.04.00 | 1.013 | 1.04 ± 1.47% | 19.11.99 | 1.04 ± 1.47% | ≥ EOL |
| 99Tc | 1.17 | 0.977 ± 0.47% | 19.11.99 | 1.39 | 1.143 ± 8.85% | 19.04.00 | 1.200 | 0.987 ± 1.94% | 19.04.00 | 0.983 ± 1.93% | ≥ EOL |
| 101Ru | 1.297 | 1.073 ± 0.30% | 19.11.99 | 1.47 | 1.214 ± 12.2% | 19.04.00 | 1.297 | 1.07 ± 1.75% | 19.11.99 | 0.983 ± 1.93% | ≥ EOL |
| 106Ru | 0.106 | 8.54E−2 ± 1.50% | 19.11.99 | 6.91E−2 | 5.73E−2 ± 14.2% | 26.01.00 | 6.91E−2* | 5.73E−2* ± 14.2% | 26.01.00 | 0.256 ± 14.2% | EOL |
| 103Rh | 0.569 | 0.471 ± 3.27% | 19.11.99 | 0.596 | 0.494 ± 4.94% | 19.04.00 | 0.575 | 0.476 ± 2.44% | 19.04.00 | 0.476 ± 2.44% | ≥ EOL |
| 109Ag | 0.128 | 0.105 ± 9.06% | 19.04.00 | 0.128 | 0.105 ± 9.06% | 19.04.00 | |||||
| 125Sb | 4.73E−3 | 3.90E−3 ± 9.43% | 26.01.00 | 4.73E−3* | 3.90E−3* ± 9.43% | 26.01.00 | |||||
| 129I | 0.279 | 0.231 ± 5.62% | 11.03.99 | 0.290 | 0.239 ± 5.62% | 24.12.99 | 0.236 ± 4.51% | ≥ EOL | |||
| 133Cs | 1.78 | 1.47 ± 1.19% | 04.05.99 | 1.68 | 1.39 ± 1.53% | 01.07.99 | 1.73 | 1.44 ± 0.94% | 01.07.99 | ||
| 134Cs | 0.154 | 0.128 ± 4.10% | 04.05.99 | 0.132 | 0.109 ± 1.53% | 01.07.99 | 0.135* | 0.221* ± 1.44% | 01.07.99 | 0.221 ± 1.43% | EOL |
| 135Cs | 0.512 | 0.424 ± 1.65% | 04.05.99 | 0.490 | 0.405 ± 1.53% | 01.07.99 | 0.499 | 0.413 ± 1.12% | 01.07.99 | 0.413 ± 1.12% | ≥ EOL |
| 137Cs | 1.91 | 1.58 ± 0.55% | 04.05.99 | 1.92 | 1.59 ± 1.52% | 01.07.99 | 1.91* | 1.65* ± 0.52% | 04.05.99 | 1.65 ± 0.52% | EOL |
| 144Ce | 8.61E−2 | 7.13E−2 ± 1.23% | 03.05.99 | 7.65E−2 | 6.32E−3 ± 1.76% | 01.07.99 | 8.29E−2* | 6.86E−2* ± 1.01% | 01.07.99 | 0.389 ± 1.00% | EOL |
| 142Nd | 3.86E−2 | 3.19E−2 ± 0.82% | 26.03.99 | 4.52E−2 | 3.73E−2 ± 5.01% | 24.11.99 | 4.52E−2 | 3.73E−2 ± 5.01% | 24.11.99 | 3.73E−2 ± 5.0% | ≥ EOL |
| 143Nd | 1.06 | 0.876 ± 1.99% | 26.03.99 | 1.14 | 0.945 ± 0.28% | 24.11.99 | 1.14 | 0.945 ± 0.28% | 24.11.99 | 0.945 ± 0.28% | ≥ EOL |
| 144Nd | 2.11 | 1.75 ± 2.00% | 26.03.99 | 2.29 | 1.89 ± 0.28% | 24.11.99 | 2.29 | 1.89 ± 0.28% | 24.11.99 | 1.89 ± 0.28% | last date |
| 145Nd | 0.993 | 0.822 ± 2.13% | 26.03.99 | 1.06 | 0.872 ± 0.28% | 24.11.99 | 1.06 | 0.872 ± 0.28% | 24.11.99 | 0.872 ± 0.28% | ≥ EOL |
| 146Nd | 1.16 | 0.958 ± 1.83% | 26.03.99 | 1.22 | 1.01 ± 0.28% | 24.11.99 | 1.22 | 1.01 ± 0.28% | 24.11.99 | 1.01 ± 0.28% | ≥ EOL |
| 148Nd | 0.596 | 0.494 ± 1.24% | 26.03.99 | 0.626 | 0.517 ± 0.29% | 24.11.99 | 0.626 | 0.517 ± 0.29% | 24.11.99 | 0.517 ± 0.29% | ≥ EOL |
| 150Nd | 0.307 | 0.254 ± 1.38% | 26.03.99 | 0.305 | 0.252 ± 0.29% | 24.11.99 | 0.305 | 0.252 ± 0.29% | 24.11.99 | 0.252 ± 0.28% | ≥ EOL |
| 147Pm | 0.17 | 0.141 ± 1.24% | 04.05.99 | 9.98E−2 | 8.52E−2 ± 9.01% | 03.03.00 | 9.98E−2* | 8.52E−2* ± 9.01% | 03.03.00 | 0.17 ± 9.00% | EOL |
| 147Sm | 0.197 | 0.163 ± 5.36% | 04.05.99 | 0.209 | 0.173 ± 0.32% | 13.12.99 | 0.209 | 0.173 ± 0.32% | 13.12.99 | 0.173 ± 0.32% | last date |
| 148Sm | 0.279 | 0.231 ± 3.78% | 04.05.99 | 0.271 | 0.224 ± 0.32% | 13.12.99 | 0.271 | 0.224 ± 0.32% | 13.12.99 | 0.224 ± 0.32% | ≥ EOL |
| 149Sm | 4.92E−3 | 4.07E−3 ± 21.4% | 04.05.99 | 3.59E−3 | 2.96E−3 ± 1.05% | 13.12.99 | 3.59E−3 | 2.96E−3 ± 1.05% | 13.12.99 | 2.96E−3 ± 1.04% | ≥ EOL |
| 150Sm | 0.476 | 0.394 ± 2.22% | 04.05.99 | 0.476 | 0.393 ± 0.32% | 13.12.99 | 0.476 | 0.393 ± 0.32% | 13.12.99 | 0.393 ± 0.32% | ≥ EOL |
| 151Sm | 1.56E−2 | 1.29E−2 ± 33.8% | 04.05.99 | 1.54E−2 | 1.27E−2 ± 0.40% | 13.12.99 | 1.54E−2* | 1.27E−2* ± 0.41% | 13.12.99 | 1.30E−2 ± 0.40% | EOL |
| 152 Sm | 0.139 | 0.115 ± 2.27% | 04.05.99 | 0.143 | 0.118 ± 0.32% | 13.12.99 | 0.143 | 0.118 ± 0.32% | 13.12.99 | 0.118 ± 0.32% | ≥ EOL |
| 154 Sm | 5.66E−2 | 4.96E−2 ± 3.73% | 04.05.99 | 6.12E−2 | 5.09E−2 ± 0.33% | 13.12.99 | 6.12E−2 | 5.09E−2 ± 0.33% | 13.12.99 | 5.05E−2 ± 0.33% | ≥ EOL |
| 151 Eu | 4.48E−4 | 3.70E−4 ± 1.05% | 01.07.99 | 4.48E−4 | 3.70E−4 ± 1.05% | 01.07.99 | |||||
| 153 Eu | 0.199 | 0.165 ± 2.1% | 04.05.99 | 0.197 | 0.162 ± 0.34% | 01.07.99 | 0.197 | 0.162 ± 0.34% | 01.07.99 | 0.162 ± 0.33% | ≥ EOL |
| 154 Eu | 3.95E−2 | 3.27E−2 ± 0.80% | 04.05.99 | 3.70E−2 | 3.06E−2 ± 2.65% | 01.07.99 | 3.92E−2* | 3.25E−2* ± 0.77% | 04.05.99 | 3.79E−2 ± 0.76% | EOL |
| 155 Eu | 1.31E−2 | 1.09E−2 ± 16.1% | 04.05.99 | 1.21E−2 | 9.97E−3 ± 4.92% | 01.07.99 | 1.21E−2* | 9.97E−3* ± 4.72% | 04.05.99 | 1.35E−2 ± 4.71% | EOL |
| 155 Gd | 4.43E−3 | 3.67E−3 ± 3.1% | 06.10.99 | 4.13E−3 | 3.41E−3 ± 1.05% | 01.12.99 | 4.19E−3 | 3.46E−3 ± 1.00% | 01.12.99 | ||
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